Thiolate gates superoxo states

Input states for quantum gates

We examine three possible implementations of nondeterministic linear optical controlled NOT gates with a view to an in-principle demonstration in the near future. To this end we consider demonstrating the gates using currently available sources, such as spontaneous parametric down conversion and coherent states, and current detectors only able to distinguish between zero and many photons. The d...

Quantum superreplication of states and gates

While the no-cloning theorem forbids the perfect replication of quantum information, it is sometimes possible to produce large numbers of replicas with vanishingly small error. This phenomenon, known as quantum superreplication, can take place both for quantum states and quantum gates. The aim of this paper is to review the central features of quantum superreplication, providing a unified view ...

Logic gates using high Rydberg states.

Connected logic gates can be operated on the levels of one molecule by making use of the special properties of high Rydberg states. Explicit experimental results for the NO molecule are provided as an example. A number of other options, including that of several gates concatenated so as to operate as a full adder, are discussed. Specific properties of high Rydberg states that are used are: thei...

Notions of local controllability for quantum gates, states and observables

Characterization of a Paramagnetic Mononuclear Nonheme Iron-Superoxo Complex

O2 bubbling into a THF solution of Fe(II)(BDPP) (1) at -80 °C generates a reversible bright yellow adduct 2. Characterization by resonance Raman and Mössbauer spectroscopy provides complementary insights into the nature of 2. The former shows a resonance-enhanced vibration at 1125 cm(-1), which can be assigned to the ν(O-O) of a bound superoxide, while the latter reveals the presence of a high-...